Aerosol Impacts on the Land-Atmosphere Interactions

 

Significance and Challenge

Atmospheric aerosols are a mixture of solid and/or liquid particles in the air, which are ubiquitous and often observable as smoke, dust, and haze [see some satellite images from NASA’s Visible Earth below]. These tiny particles can have a variety of important impacts on the environment. Sulfate, nitrate, and some other ions in the aerosols are a major source of acid precipitation. In addition, fine particles may have a significant detrimental effect on human health. This concern has led to proposals to reduce concentration of fine particles by emissions control. The atmospheric deposition of mineral dust containing iron may alter the marine biological activity.

Through their scattering and absorption of radiation (so-called direct effect), aerosols can also induce some other important environment effects. For example, aerosols are a major contributor to visibility problem in urban centers as well as rural areas. Closely related to the visibility problem is the scattering and absorption of solar UV by aerosols that can have significant impacts on both the DNA damaging UV radiation reaching the surface [Liu et al., 1991] and photochemistry in the boundary layer [Dickerson et al., 1997]. Aerosols can also have significant impacts on the ecological system [Chameides et al., 1999]. Finally and probably most importantly, tropospheric aerosols are believed to play a significant role in the earth's energy budget and climate through the direct effect [Coakley et al., 1983; Charlson et al., 1992; Penner et al., 1992] as well as altering cloud microphysical and optical properties (so-called indirect effect) [Twomey, 1977; Albrecht, 1989]. The radiative forcing of anthropogenic aerosols may be comparable to that of greenhouse gases but with the opposite sign [IPCC, 2001].

In the past two decades, considerable research efforts and significant scientific progress have been made. On the other hand, large uncertainties exist in the current estimates of aerosol forcing because of incomplete knowledge concerning the physical and chemical properties of the aerosols, their global/regional distributions, and the aerosol-cloud interactions. Even less studied is how the atmosphere responds to the aerosol radiative perturbations at the surface and in the atmosphere, which should depend on land cover and large-scale motion (e.g., mid-latitude subsidence vs. tropical ascending). Quantification of potential impacts of aerosols on ecological system and biogenic emissions remains challenging. 

Research Topics and Approaches

Aerosol research in our group dates back to more than ten years ago. In 1992, Prof. Dickinson coauthored a Science paper with Profs. Penner and O’Neill that estimates effects of biomass burning aerosol on global radiation budget. Currently under the auspices of NSF, DOE, and NASA, the group is addressing several outstanding scientific questions on both regional and global scale, by using satellite remote sensing of aerosols, land surface properties, cloud and precipitation (e.g., MODIS, TOMS, TRMM, CERES, ISCCP, etc.), and conducting both one-dimensional (1-D) and three-dimensional (3-D) modeling of atmosphere-land interactions. Some activities are conducted in collaboration with Prof. Fu’s and Prof. Chameides groups. Specifically, our current research topics include:

         Characterization of regional/global aerosol distributions using the assimilation approach

         Quantification of aerosol solar radiative forcing and its impacts on the biosphere

         Exploration of aerosol impacts on the land-atmosphere interactions and climate

Related Publications

        Yu, Hongbin, R.E. Dickinson, M. Chin, Y.J. Kaufman, M. Zhou, L. Zhou, Y. Tian, O. Dubovik, and B.N. Holben (2004), The direct radiative effect of aerosols as determined from a combination of MODIS retrievals and GOCART simulations, J. Geophys. Res., 109, D03206, doi:10.1029/2003JD003914. reprint (pdf) [Copyright 2003 American Geophysical Union. Further reproduction or electronic distribution is not permitted.]

 

 Yu, Hongbin, R.E. Dickinson, M. Chin, Y.J. Kaufman, B.N. Holben, I.V. Geogdzhayev, and M.I. Mishchenko: Annual cycle of global distributions of aerosol optical depth from integration of MODIS retrievals and GOCART model simulations. Journal of Geophysical Research, 108 (D3), 4128, doi:10.1029/2002JD002717, 2003. reprint (pdf), color figures (ps files) [Copyright 2003 American Geophysical Union. Further reproduction or electronic distribution is not permitted.]

 

 Yu, Hongbin, S.C. Liu, and R.E. Dickinson: Radiative effects of aerosols on the evolution of the atmospheric boundary layer. Journal of Geophysical Research, 107 (D12), 4142, doi:10.1029/2001JD000754, 2002.  reprint (pdf) [Copyright 2002 American Geophysical Union. Further reproduction or electronic distribution is not permitted.] 

 Liu, Y.Q., S.C. Liu, R.E. Dickinson: Regional response of atmospheric circulation and surface energy and water balance to observed distribution of aerosol loading over the United States, Journal of Climate (in review). 

  Yu, Hongbin, Radiative Effects of Aerosols on the Environment in China, Ph.D. Dessertation, 226pp, School of Earth and Atmospheric Sciences, Georgia Institute of Technology, July 2000.

 Chameides W.L., H. Yu, S.C. Liu, M. Bergin, X. Zhou, L. Mearns, W. Gao, C.S. Kiang, R. Saylor, Chao Luo, Yan Huang, A. Steiner, and F. Giorgi: A case study of the effect of atmospheric aerosols and regional haze on agriculture: An opportunity to enhance crop yields in China through emission controls? Proceedings of the National Academy of Sciences of the United States of America (PNAS), 96 (24), 13626-13633, 1999.

 Penner, J.E., R. E. Dickinson, C.A. O'Neill: Effects of aerosol from biomass burning on the global radiation budget, Science, 256, 1432-1434, 1992.

Presentations

 Yu, Hongbin, Yan Zhang, R.E. Dickinson, Rong Fu, Simulations of smoke-land-atmosphere interactions over forest and pasture, AGU 2003 Fall meeting, San Francisco, December 8-12, 2003.  

 Zhou, Mi, Hongbin Yu, and R.E. Dickinson: Application of MODIS land albedo to estimate of aerosol direct radiative forcing, Solar Radiation and Climate Gordon Conference, July 13-18, 2003, New London, NH.

 Yu, Hongbin: Impacts of aerosols on the land-air interactions. NASA Goddard Space Flight Center, AEROCENTER, Greenbelt, Maryland, March 20, 2002.

 Yu, Hongbin, S.C. Liu, and R.E. Dickinson: Radiative effects of aerosols on the evolution of the atmospheric boundary layer. EOS Trans., AGU 2001 Spring Meeting, A51B-03, Boston, Mass., May 29 – June 2, 2001.

 

Sponsors

 Office of Science (Biological and Environment Research), the U.S. Department of Energy (DOE)

 Atmospheric Science Division, the U.S. National Science Foundation (NSF)

 AEROCENTER Visiting Scientist Program, National Aeronautics and Space Administration (NASA)

 

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