Exploration of Aerosol Impacts on the Land-Atmosphere Interactions and Climate

Aerosols heat the atmosphere through absorption and cool the land surface even more through scattering and absorption. A figure shown here is an example that the dry-season biomass burning aerosol in the southern hemispheric tropics heats the atmosphere and cools the surface substantially. As suggested by our radiative calculations, about a half of surface cooling is compensated by the atmospheric heating globally. Such perturbation and redistribution of energy will influence atmospheric stratification, turbulent mixing, atmosphere-surface interaction, and atmospheric circulation. Our objectives are to examine (1) how aerosols affect the surface energy balance and its partitioning into sensible heat flux and evapotranspiration (ET); (2) how the changes in ABL temperature and moisture feedback such partitioning; (3) how the evolution of the ABL is influenced by the changes in surface heating and entrainment at the top of  the ABL; (4) how the aerosol-land interactions depend on land cover and atmospheric conditions; and (5) how aerosol’s regulation on the partitioning of ET into different time scale fluxes, namely canopy transpiration, canopy evaporation, and ground evaporation, consequently correlates with convective precipitation, circulation patterns, and the overall hydrological cycle.

To achieve these goals, we are employing both 1-D and 3-D models to examine such impacts, focusing on its diurnal cycle. Although perhaps unrealistic in some aspects, 1-D models provide high resolution and flexibility in conducting sensitivity studies, allowing the atmospheric response to radiative perturbations to be examined more easily than possible with complex 3-D models, thus complementing and facilitating the interpretation of 3-D model results.

A high-resolution ABL model has been used to investigate the impacts of aerosols on the evolution of the ABL for dry subsiding regions [Yu et al., 2002]. It shows that tropospheric aerosols have substantial effects on land surface processes including temperatures and latent fluxes that for absorbing aerosols are largely unconnected with TOA radiative forcing. In particular, aerosols affect the ET through reducing the solar radiation reaching the surface and changing the entrainment at the top of the ABL, depending on the loading, absorption, and vertical profile of aerosols, as well as soil moisture. We are extending our study to tropical ascending regions using the NCAR SCCM, a single-column version of NCAR CCM3. We examine how absorbing aerosol perturbs the diurnal cycle of cloud, atmospheric stratification, surface fluxes, and convection and what controls of land cover exert on such impacts. 

We have also used NCAR regional climate model at a 60km horizontal resolution, namely RegCM, to examine how aerosols affect the land surface energy, water balance, and atmospheric circulation in the US [Liu et al., 2001]. The annual cycle of global aerosol distribution derived from MODIS retrievals and GOCART simulations is being incorporated into RegCM and the newly released CCSM to explore the role of aerosols in changing atmospheric circulation and climate.

            These modeling activities have also inspired us to analyze climatology data for fingerprints of aerosol impacts on climate. The 22-year TOMS data show that the magnitude and duration of biomass burning aerosol vary interannually over Amazon (0-20S, 40-70W), which can be correlated with the deviations of wet season onsets from their climatological mean (the positive numbers of pentads represent delayed onset and negative numbers for early onset). In collaboration with Prof. Fu’s group and through a combination of multiple data sets (e.g., ISCCP, TRMM, CERES, TOMS, MODIS, and others), we are examining (1) how biomass burning smoke would affect the land surface processes and modify the atmospheric boundary conditions needed for the onset of wet season over South American Monsoon region, and (2) how such effects interact with the influence of large-scale circulation anomalies.